瞿赞(Qu Zan)
研究员
电子邮件:quzan(a)sjtu.edu.cn
办公室电话:02154745591
办公地点:57365线路检测中心闵行校区环境科学楼1031室
团队网页:http://air.sjtu.edu.cn/
研究方向
- 大气污染控制技术
- 重金属控制技术
- 便携式烟气净化工艺与装备
个人简历
1995.09-1999.07,毕业于郑州大学化工学院,获得学士学位;
1999.09-2002.07,毕业于郑州大学化工学院,获得硕士学位;
2003.03-2007.04,毕业于57365线路检测中心,获得博士学位;
2007.04-2008.03, 美国加州大学劳伦斯-伯克利国家实验室,博士后;
2008.03-2011.12, 57365线路检测中心,讲师;
2012.01-2016.12, 57365线路检测中心,副教授;
2015.09-2016.09, 美国佐治亚理工学院,访问学者;
2017.01-至今,57365线路检测中心,研究员。
研究论文
- Qu, Z.; Yan, N.Q.*; Zhao, Y.F.; Jia, J.P.; Wu, D. Removal of dibenzothiophene from the simulated petroleum by gamma-irradation induced reaction. Energy Fuels, 2006, 20, 142-147.
- Qu, Z.; Yan, N.Q.*; Jia, J.P.; Wu, D. Removal of dibenzothiophene from simulated petroleum by integrated gamma-irradiation and Zr/alumina catalyst. Applied Catalysis B: Environmental. 2007, 71, 108-115.
- Qu, Z.; Yan N.Q.*; Liu, P.; Chi, Y.; Jia, J.P. Bromine chloride as an oxidant to improve elemental mercury removal from coal-fired flue gas. Environmental Science Technology. 2009, 43, 8610-8615.
- Qu, Z.; Chang, J.J.; Hsiung, T.L.; Yan, N.Q.; Wang, H.P.; Dod, R.; Chang, S.G.*; Miller, C. Halides on Carbonaceous Materials for Enhanced Capture of Hg0: Mechanistic Study. Energy Fuels. 2010, 24, 3534-3539.
- Qu, Z.; Yan, N.Q.*; Liu, P.; Jia, J.P.; Yang, S.J. The role of iodine monochloride for the oxidation of elemental mercury. Journal of Hazardous Materials. 2010, 183(1-3), 132-137.
- Qu, Z.; Yan N.Q.*; Liu, P.; Guo, Y.F.; Jia, J.P. Oxidation and stabilization of elemental mercury from coal-fired flue gas by sulfur monobromide. Environmental Science Technology. 2010, 44, 3889-3894.
- Yan, N.Q.*; Chen, W.M.; Chen, J.; Qu, Z.*; Guo, Y.F.; Yang, S.J.; Jia, J.P. Significance of RuO2 Modified SCR catalyst for elemental mercury oxidation in coal-fired flue gas. Environmental Science Technology. 2011, 45, 5725-5730.
- Xie, J.K.; Qu, Z.*; Yan, N.Q.*; Yang, S.J.; Chen, W.M.; Hu, L.G.; Huang, W.J.; Liu, P. Novel regenerable sorbent based on Zr–Mn binary metal oxides for flue gas mercury retention and recovery. Journal of Hazardous Materials. 2013, 261, 206-213.
- Xie, J.K.; Xu, H.M.; Qu, Z.*; Huang, W.J.; Chen, W.M.; Ma, Y.P.; Zhao, S.J.; Liu, P.; Yan, N.Q.* Sn–Mn binary metal oxides as non-carbon sorbent for mercury removal in a wide-temperature window. Journal of Colloid and Interface Science. 2014, 428, 121-127.
- Chen, W.M.; Ma, Y.P.; Yan, N.Q.*; Qu, Z.*; Yang, S.J.; Xie, J.K.; Guo, Y.F.; Hu, L.G.; Jia, J.P. The co-benefit of elemental mercury oxidation and slip ammonia abatement with SCR-Plus catalysts. Fuel. 2014, 133, 263-269.
- Ma, Y.P.; Xu, H.M.; Qu, Z.*; Yan, N.Q.*; Wang, W.H. Absorption characteristics of elemental mercury in mercury chloride solutions. Journal of Environmental Sciences. 2014, 2257-2265.
- Chen, W.M.; Ma, Y.P.; Qu, Z.*; Liu, Q.H.; Huang, W.J.; Hu, X.F.; Yan, N.Q.* Mechanism of the Selective Catalytic Oxidation of Slip Ammonia over Ru-Modified Ce−Zr Complexes Determined by in Situ Diffuse Reflectance Infrared Fourier Transform Spectroscopy. Environmental Science Technology. 2014, 48, 12199-12205.
- Ma, Y.P.; Qu, Z.*; Xu, H.M.; Wang, W.H.; Yan, N.Q. Investigation on mercury removal method from flue gas in the presence of sulfur dioxide. Journal of Hazardous Materials. 2014, 279, 289-295.
- Qu, Z.; Yan, L.L.; Li, L.*; Xu, J.F.; Liu, M.M.; Li, Z.C.; Yan, N.Q.* Ultraeffective ZnS nanocrystals sorbent for mercury (II) removal based on size-dependent cation exchange. ACS Applied Materials Interfaces. 2014, 6, 18026-18032.
- Xu, H.M.; Xie, J.K.; Ma, Y.P.; Qu, Z.*; Zhao, S.J.; Chen, W.M.; Huang, W.J.; Yan, N.Q.* The cooperation of Fe-Sn in a MnOx complex sorbent used for capturing elemental mercury. Fuel. 2015, 140, 803-809.
- Zhao, S.J.; Qu, Z.*; Yan, N.Q.*; Li, Z.; Zhu, W.F.; Pan, J.; Xu, J.F.; Li, M.D. Ag-modified AgI-TiO2 as an excellent and durable catalyst for catalytic oxidation of elemental mercury. RSC Advances. 2015, 5, 30841-30850.
- Xu, H.M.; Qu, Z.*; Huang, W.J.; Mei, J.; Chen, W.M.; Zhao, S.J.; Yan, N.Q. Regenerable Ag/graphene sorbent for elemental mercury capture at ambient temperature. Colloids and Surfaces A: Physicochemical and Engineering Aspects. 2015, 476, 83-89.
- Ma, Y.P.; Xu, H.M.; Qu, Z.*; Yan, N.Q.; Wang, W.H. Removal of mercury from flue gas from nonferrous metal smelting, by use of mercury chloride solution, and mechanisms of inhibition by sulfur dioxide. Research on Chemical Intermediates. 2015, 41, 5889-5905.
- Xu, H.M.; Qu, Z.*; Zong, C.X.; Huang, W.J.; Quan, F.Q.; Yan, N.Q.* MnOx/graphene for the catalytic oxidation and adsorption of elemental mercury. Environmental Science Technology. 2015, 49, 6823-6830.
- Qu, Z.; Xie, J.K.; Xu, H.M.; Chen, W.M.; Yan, N.Q.* Regenerable sorbent with a high capacity for elemental mercury removal and recycling from the simulated flue gas at a low temperature. Energy Fuels. 2015, 29(10), 6187-6196.
- Huang, W.J.; Xu, H.M.; Qu, Z.*; Zhao, S.J.; Chen, W.M.; Yan, N.Q.* Significance of Fe2O3 modifed SCR catalyst for gas-phase elemental mercury oxidation in coal-fired flue gas. Fuel Processing Technology. 2016, 149, 23-28.
- Huang, W.J.; Qu, Z.*; Chen, W.M.; Xu, H.M.; Yan, N.Q.* An enhancement method for the elemental mercury removal from coal-fired flue gas based on novel discharge activation reactor. Fuel. 2016, 171, 59-64.
- Xu, J.F.; Qu, Z.*; Yan, N.Q.; Zhao, Y.X.; Hu, X.F.; Li, L.* Size-dependent nanocrystal sorbent for copper removal from water. Chemical Engineering Journal. 2016, 284, 565-570.
- Zhu, Z.X.; Ma, Y.P.; Qu, Z.*; Fang, L.; Zhang, W.Y.; Yan, N.Q. Study on a new wet flue gas desulfurization method based on the Bunsen reaction of sulfur-iodine thermochemical cycle. Fuel. 2017, 195, 33-37.
- Qu, Z.*; Fang, L.; Chen, D.Y.; Xu, H.M.; Yan, N.Q. Effective and regenerable Ag/graphene adsorbent for Hg(II) removal from aqueous solution. Fuel. 2017, 203, 128-134.
- Chen, D.Y.; Zhao, S.J.*; Qu, Z.*; Yan, N.Q. Cu-BTC as a novel material for elemental mercury removal from sintering gas. Fuel. 2018, 217, 297-305.
- Fang, L.; Li, L.; Qu, Z.*; Xu, H.M.; Xu, J. F.; Yan, N.Q. A novel method for the sequential removal and separation of multiple heavy metals from wastewater. Journal of Hazardous Materials. 2018, 342, 617-624.
- Quan, Z.W.; Huang, W.J.; Liao, Y.; Liu, W.; Xu, H.M.; Yan, N.Q.; Qu, Z.* Study on the regenerable sulfur-resistant sorbent for mercury removal from nonferrous metal smelting flue gas. Fuel. 2019, 241, 451-458.
- Liao, Y.; Xu, H.M.; Liu, W.; Ni, H.F.; Zhang, X.G.; Zhai, A.P.; Quan, Z.W.; Qu, Z.*; Yan, N.Q. One step interface activation of ZnS using cupric ions for mercury recovery from nonferrous smelting flue gas. Environmental Science Technology. 2019, 53, 4511-4518.
- Liu, W.; Zhou, Y.X.; Hua, Y.F.; Peng, B.; Deng, M.; Yan, N.Q.; Qu, Z.* A Sulfur-resistant CuS-modified active coke for mercury removal from solid waste incineration flue gas. Environmental Science and Pollution Research. 2019, 26, 24831-24839.
- Li, J.X.; Xu, H.M.; Liao, Y.; Qiu, Y.X.; Yan, N.Q.; Qu, Z.* Atomically Dispersed Manganese on a Carbon-Based Material for the Capture of Gaseous Mercury: Mechanisms and Environmental Applications. Environmental Science Technology. 2020, 54(8), 5249-5257.
- Wang, L.L.; Xu, H.M.; Qiu, Y.X.; Liu, X.S.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Utilization of Ag nanoparticles anchored in covalent organic frameworks for mercury removal from acidic waste water. Journal of Hazardous Materials. 2020, 389, 121824.
- Liu, W.; Xu, H.M.; Liao, Y.; Wang, Y.L.; Yan, N.Q.; Qu, Z.* Co-doped ZnS with large adsorption capacity for recovering Hg0 from non-ferrous metal smelting gas as a co-benefit of electrostatic demisters. Environmental Science and Pollution Reserach. 2020, 27, 20469–20477.
- Mei, J.; Liao, Y.; Qin, R.Y.; Sun, P.X.; Wang, C.; Ma, Y.P.; Qu, Z.*; Yan, N.Q.; Yang, S.J.* Acceleration of Hg0 adsorption onto natural sphalerite by Cu2+ activation during flotation: mechanism and applications in Hg0 recovery. Environmental Science Technology. 2020, 54, 7687-7696.
- Liao, Y.; Liu, W.; Xu, H.M.; Hong, Q.Y.; Wang, Y.L.; Qu, Z.*; Yan, N.Q. Zinc concentration internal circulation technology for elemental mercury recovery from zinc smelting flue gas. Fuel. 2020, 280, 118566.
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Wang, L.L.; Deng, M.; Xu, H.M.; Li, W.W.; Huang, W.J.; Yan, N.Q.; Zhou, Y.X.; Chen, J.S.; Qu, Z.* Selective reductive removal of silver ions from acidic solutions by redox-active covalent organic frameworks. ACS Applied Materials & Interfaces. 2020, 12, 37619-37627.
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Sun, Y.N.; Deng, M.; Huang, W.J.; Zhou, Y.X.; Zhao, Y.; Chen, J.S.; Yan, N.Q.; Qu, Z.* Radical-Induced Oxidation Removal of Mercury by Ozone Coupled with Bromine. ACS ES&T Engineering. 2021, 1, 110-116.
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Sun, Y.N.; Xie, J.K.; Huang, W.J.; Li, G.; Li, S.C.; Cui, P.; Xu, H.M.; Qu, Z.*; Yan, N.Q. Novel product-adjustable technology using Wellman-Lord method coupled with sodium-alkali for SO2 removal and regeneration from smelting gas. Fuel. 2021, 288, 119714.
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Wang, L.L.; Zhang, K.; Luo, J.M.; Ma, J.Y.; Ji, W.X.; Hong, Q.Y.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Metastable Facet-Controlled Cu2WS4 Single Crystals with Enhanced Adsorption Activity for Gaseous Elemental Mercury. Environmental Science Technology. 2021, 55, 5347-5356.
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Li, J.X.; Xu, H.M.; Huang, Z.J.; Hong, Q.Y.; Qiu, Y.X.; Yan, N.Q.; Qu, Z.* Strengthen the affinity of element mercury on the carbon-based material by adjusting the coordination environment of single-site manganese. Environmental Science Technology. 2021, 55, 14126−14135.
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Xu, H.M.; Hong, Q.Y.; Li, J.X.; Liao, Y.; Huang, W.J.; Qu, Z.*; Yan, N.Q. Heterogeneous Reaction Mechanisms and Functional Materials for Elemental Mercury Removal from Industrial Flue Gas. ACS ES&T Engineering. 2021, 1, 10, 1383–1400.
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Wang, L.L.; Ji, L.P.; Li, W.W.; Zhang, K.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Fabrication of Cu2S hollow nanocages with enhanced high-temperature adsorption activity and recyclability for elemental mercury capture. Chemical Engineering Journal. 2022, 427, 130935.
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Huang, W.J.; Xu, H.M.; Liu, X.S.; Wang, L.L.; Li, S.T.; Ji, L.P.; Qu, Z.*; Yan, N.Q. Surface protection method for the magnetic core using covalent organic framework shells and its application in As(III) depth removal from acid wastewater. Journal of Environmental Sciences, 2022, 115, 1-9.
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Li, W.W.; Gao, G.Q.; Wang, L.L.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Dual confinement strategy based on metal-organic frameworks to synthesize MnOx@ZrO2 catalysts for toluene catalytic oxidation. Fuel, 2022, 320, 123983.
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Gao, G.Q.; Liao, Y.; Li, W.W.; Li, Z.H.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Active Surface RuOx Species Originating from Size-Driving Self-Dispersion Process for Toluene Catalytic Combustion. Chemical Engineering Journal, 2022, 441, 136127.
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Wang, L.L.; Zhang, K.; Li, J.X.; Shen, X.R.; Yan, N.Q.; Zhao, H.Z.; Qu, Z.* Engineering of Defect-Rich Cu2WS4 Nano-homojunctions Anchored on Covalent Organic Frameworks for Enhanced Gaseous Elemental Mercury Removal. Environmental Science Technology. 2022, 56, 22, 16240-16248.
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Huang, W.J.; Zong, C.X.; Liu, Z.S.; Hong, Q.Y.; Ji, L.P.; Xu, H.M.; Qu, Z.*; Yan, N.Q. Cubic SAPO-34 supported MnOx for low-temperature gaseous mercury oxidation and adsorption from coal-fired flue gas. Fuel. 2023, 332, 126142.
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Li, W.W.; Liu, Z.S.; Wang, L.L.; Gao, G.Q.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Wang, H.W.; Qu, Z.* FeSx@MOF-808 composite for efficient As(III) removal from wastewater: behavior and mechanism. Journal of Hazardous Materials. 2023, 446, 130681.
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Li, J.X.; Li, H.L.; Xu, H.M.; Hong, Q.Y.; Ji, L.P.; Liu, Z.S.; Qiu, Y.X.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake. Biochar. 2023, 5(13).
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Xu, H.M.; Hong, Q.Y.; Zhang, Z.Y.; Cai, X.L.; Fan, Y.R.; Liu, Z.S.; Huang, W.J.; Yan, N.Q.; Qu, Z.*; Zhang, L.Z.* SO2-Driven In Situ Formation of Superstable Hg3Se2Cl2 for Effective Flue Gas Mercury Removal. Environmental Science Technology. 2023, 57, 13, 5424-5432.
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Chen, C.; Huang, W.J.; Xu, H.M.; Liu, Z.S.; Li, X.W.; Shi, H.Z.; Yu, Y.M.; Qu Z.*; Yan, N.Q. CO2 sequestration and CaCO3 recovery with steel slag by a novel two-step leaching and carbonation method. Science of the Total Environment. 2023, 891, 164203.
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Gao, G.Q.; Liu, W.; Liu, Z.S.; Li, Z.H.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Electron Donation from Boron Suboxides via Strong p–d Orbital Hybridization Boosts Molecular O2 Activation on Ru/TiO2 for Low-Temperature Dibromomethane Oxidation. Environmental Science Technology. 2023, 57, 45, 17566-17576.
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Liu, Z.S.; Xu, H.M.; Fan, Y.R.; Hong, Q.Y.; Huang, W.J.; Yu, F.; Qu, Z.*; Yan, N.Q. Cation Concavities Induced d-Band Electronic Modulation on Co/FeOx Nanostructure to Activate Molecular and Interfacial Oxygen for CO Oxidation. Environmental Science Technology. 2023, 57, 50, 21272-21283.
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Li, W.W.; Cheng, C.; Gao, G.Q.; Xu, H.M.; Huang, H.M.; Qu, Z.*; Yan, N.Q. Trace SO2 capture within the engineered pore space using a highly stable SnF62−-pillared MOF. Material Horizons. 2024, 11, 8, 1889-1898.
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Xie, Y.B.; Wang, X.Q.*; Qu, Z.*; Ning, P.*; Wang, L.L.; Xu, H.M.; Huang, W.J.; Lu, J.C.; Luo, J.F. Enhancing AsH3 Detoxification via Electron-Deficient [NiIII-OH (μ-O)] in a Nickel-Modified NaY Zeolite: A Pathway toward As0 Products. Environmental Science Technology. 2024, 58, 15, 6704-6715.
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Hong, Q.Y.; Xu, H.M.*; Sun, X.M.; Li, J.X.; Huang, W.J.; Qu, Z.*; Zhang, L.Z.; Yan, N.Q.* In-situ low-temperature sulfur CVD on metal sulfides with SO2 to realize self-sustained adsorption of mercury. Nature Communications. 2024, 15, 3362.
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Liu, Z.S.; Fan, Y.R.; Xu, H.M.; Huang, W.J.; Yu, F.; Qu, Z.*; Yan, N.Q. Asymmetric Coordination of Single-Atom Ru Sites Achieves Efficient N(sp3)-H Dehydrogenation Catalysis for Ammonia Oxidation. Environmental Science Technology. 2024, 58, 24, 10717-10728.
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Fan, Y.R.; Xu, H.M.*; Gao, G.Q.; Wang, M.M.; Huang, W.J.; Ma, L.; Yao, Y.C.*; Qu, Z.*; Xie, P.F.*; Dai, B.; Yan, N.Q. Asymmetric Ru-In atomic pairs promote highly active and stable acetylene hydrochlorination. Nature Communications. 2024, 15, 6035.
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Fan, Y.R.; Wang, M.M.; Liu, Z.S.; Gao, G.Q.; Hong, Q.Y.; Huang, W.J.; Ma, L.; Qu, Z.*; Yan, N.Q.; Xu, H.M.*Lattice-Strain Engineering in Ni–Ru Heterostructures for Efficient Acetylene Hydrochlorination toward Vinyl Chloride. ACS Nano. 2024, 18, 31, 20624-20635.
科研项目
一、国家自然科学基金委项目
1. 国家自然科学基金(青年项目),弱电离环境中卤硫化物对烟气零价汞的去除机制研究,50908145,2010.01-2012.12,项目负责人;
2. 国家自然科学基金(面上项目),含溴除汞促进剂在烟气除汞过程中的归趋及其次生污染控制研究,51278294,2013.01-2016.12,项目负责人;
3. 国家自然科学基金(面上项目),有色金属冶炼烟气汞定向形态调控回收技术原理研究,21677096,2017.01-2020.12,项目负责人;
4. 国家自然科学基金(面上项目),基于高温过滤/催化体系协同脱除焚烧烟气持久性有机污染物与汞的应用基础研究,52070129,2021.01-2024.12,项目负责人;
5. 国家自然科学基金(面上项目),构效精确匹配的复合型钌基催化材料用于溴代烃去除的应用基础研究,52470123,2025.01 - 2028.12,项目负责人;
6. 国家自然科学基金(重点项目),TMS功能材料的绿色制备及其在烟气硫/汞低碳协同控制中的应用研究,22436004,2025.01 - 2029.12,项目骨干(排名第2);
二、科技部项目
1. 国家高技术研究发展计划项目(863计划),燃煤锅炉烟气汞污染排放控制技术,2007AA06Z340,2007-2010,子课题负责人;
2. 国家高技术研究发展计划项目(863计划),工业锅炉湿法脱硫脱硝脱汞技术与示范,2011AA060801,2011-2014,子课题负责人;
3. 国家高技术研究发展计划项目(863计划),有色炉窑烟气高浓度SO2回收及重金属协同控制技术研究与示范, 2012AA062504,2012-2014,子课题负责人;
4. 国家重点基础研究发展计划项目(973计划),汞污染排放过程形态调控机制及控制技术原理,2013CB430005,2013-2017,子课题负责人;
5. 国家重点研发计划项目,有色金属冶炼烟气多污染物协同控制技术,2017YFC0210500,2017-2020,子课题负责人;
6. 国家重点研发计划项目,高原高寒地区灾害现场安置装备关键技术与装备研究及应用示范,2017YFC0806300,2017-2020,子课题负责人;
7. 生态环境部对外合作中心"中国履行《关于汞的水俣公约》能力建设项目",四川省有色金属冶炼行业含汞废物环境无害化管理现状评估,FECO/LY4/S/22/013,2021-2022,课题负责人。
荣获奖项
- 57365线路检测中心优秀共产党员,2011年;
- 57365线路检测中心“SMC-晨星青年学者”奖励计划(B类),2012年;
- 57365线路检测中心“晨星-优秀学者"奖励计划(教授A类),2018年;
- 《燃煤烟气汞及其它污染物协同控制技术研发与应用》,教育部技术发明二等奖,2018年;
- 《铁基尖晶石材料用于协同除汞脱硝的应用基础研究》,上海市自然科学二等奖,2018年;
- 《有色金属冶炼行业污酸处理及资源化利用关键技术》,河南省教育厅科技成果一等奖,2019年;
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《有色金属冶炼行业污酸处理及资源化利用关键技术》,河南省科技进步三等奖,2020年;
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《疫情医疗废物应急处置装置研发与应用》,中国发明协会发明创业成果一等奖,2020年;
- 57365线路检测中心优秀共产党员,2021年;
- 《我国汞污染特征、环境过程及减排技术原理》,贵州省自然科学一等奖,2021年。
- 《燃煤烟气硫-硝-汞联合脱除关键技术研究》,中华环保联合会科技进步二等奖,2022年。
- 《有色冶炼烟气多污染物协同控制耦合资源化技术与应用》(发明),中国有色金属工业科学技术一等奖,2022年。
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《有色金属冶炼烟气多污染物协同控制技术研发与应用》,教育部技术发明一等奖,2022年。
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《工业烟气超低排放与协同控制关键材料及技术装备》,浙江省科技进步一等奖,2022年。